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              <p>Arc lavas display elevated Fe31/RFe ratios relative to MORB. One mechanism to explain this isthe mobilization and transfer of oxidized or oxidizing components from the subducting slab to the mantlewedge. Here we use iron and zinc isotopes, which are fractionated upon complexation by sulfide, chloride,and carbonate ligands, to remark on the chemistry and oxidation state of fluids released during progrademetamorphism of subducted oceanic crust. We present data for metagabbros and metabasalts from theChenaillet massif, Queyras complex, and the Zermatt-Saas ophiolite (Western European Alps), which havebeen metamorphosed at typical subduction zone P-T conditions and preserve their prograde metamorphichistory. There is no systematic, detectable fractionation of either Fe or Zn isotopes across metamorphicfacies, rather the isotope composition of the eclogites overlaps with published data for MORB. The lack ofresolvable Fe isotope fractionation with increasing prograde metamorphism likely reflects the mass balanceof the system, and in this scenario Fe mobility is not traceable with Fe isotopes. Given that Zn isotopes arefractionated by S-bearing and C-bearing fluids, this suggests that relatively small amounts of Zn are mobilizedfrom the mafic lithologies in within these types of dehydration fluids. Conversely, metagabbros fromthe Queyras that are in proximity to metasediments display a significant Fe isotope fractionation. Thecovariation of d56Fe of these samples with selected fluid mobile elements suggests the infiltration of sedimentderived fluids with an isotopically light signature during subduction.</p>
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